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Long Island, according to Wikipedia, is the largest "in the contiguous United States", however biggest in the us (as written in the question) is Hawaii "With an area of 4,028 square miles (10,430 km2)". Prior to Long Island are nine islands in Alaska and all of Puerto Rico.

http://en.wikipedia.org/wiki/List_of_islands_of_the_United_States_by_area

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