Sussex County.
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Mecklenburg County is the second largest county in North Carolina, in terms of population and size. It is home to the city of Charlotte, which is the largest city in the state.
San Bernardino County in California is the largest county in the United States by size. It covers approximately 20,105 square miles.
The largest county in the UK is North Yorkshire, covering an area of approximately 3,341 square miles.
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