Two things rate as the largest origami structures.
A 81.94 m [268 ft 10 in] crane was constructed 2009 in Hiroshima, Japan as part of the Peace Piece Project.
The longest project was a 649 m (2128 ft) catepillar in Germany 2004. It took 60 people 60 hours and 25,000 sheets of paper to make this big bug.
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The largest of the seven wonders of the ancient world is believed to be the Great Pyramid of Giza. It is the oldest and only structure still intact today.
The largest structure is the Great Wall. The largest category of "stuff" is dark energy.
IN 1999, the portable structure or tent which is called 'Tensile 1' was awarded the 'Worlds Largest Portable Event Venue'. The structure has a surface area of nearly 14,000 square metres or 150,000 square feet in one structure, ie not lots of smaller structures joined together. (Guinness World Records, (1999) Guinness Superlatives, London).
The largest structure in an animal cell is the nucleus. It houses genetic material (DNA) and controls the cell's activities.
The Great Wall of China is considered one of the biggest superstructures in the world, stretching over 13,000 miles.